This is a collection of input files, output files, and scripts, which were used to produce all the data reported in the following publication: "Nonlinear quantum magnetophononics in SrCu2(BO3)2" Flavio Giorgianni, Björn Wehinger, Stephan Allenspach, Nicola Colonna, Carlo Vicario, Pascal Puphal, Ekaterina Pomjakushina, Bruce Normand, Christian Rüegg arXiv:2101.01189 Calculations were performed using the Quantum ESPRESSO (QE) distribution. The following codes of Quantum ESPRESSO were used: pw.x - self-consistent-field ground-state calculation using density-functional theory (DFT) or Hubbard-corrected DFT (DFT+U); ph.x - density functional perturbation thoery at PBE level for the calculation of Born Effective charges CONTENT OF FOLDERS: PBE |** RELAX (folder containing files for the calculation of the DFT equilibrium structure) | |- pwscf.in, pwscf.out - input/output files for pw.x | |- final_pos.xsf - xsf file with equilibrium geometry | |- job.sh - submission script | |** BORN_eff_CHARGES (folder containing files for the calculation of the Born effective charges) | |- pwscf.in, pwscf.out - input/output files for pw.x | |- phscf.in, phscf.out - input/output files for ph.x | |- job.sh - submission script | PBE_plus_U |** RELAX (folder containing files for the calculation of the DFT+U equilibrium structure) | |- pwscf.in, pwscf.out - input/output files for pw.x | |- final_pos.xsf - xsf file with equilibrium geometry | |- job.sh - submission script | |** Exc_PARAMETERS (folder containing the files for the calculation of the exchage parameters) | |** Equilibrium | | |** Conf* (*=1,2,3,4) (4 different spin configurations needed for the exchange parameters calculation) | | | |- pwscf.in, pwscf.out - input/output files for pw.x | | | |- struct_mag.xsf - xsf file with the geometrical and magnetic structure | | | |- job.sh - submission script | | | | | |- Cu_mag_configs.txt - txt file with the different spin orientation for the 8 Cu atoms in the | | | primitive AFM cell for each spin configurations 1-4 | | |- exch.sh - bash script to compute the J parameters | | | |** PHONON_4.60THz | | |** Conf* (*=1,...,11) (11 different spin configurations in the phonon-distorted 2x2x1 supercell needed for the calculation of the | | | | independent J parameters) | | | |** amplitude* (*=-0.2, ..., 0.2) (different strenght of the displacement along the phonon mode) | | | | |- pwscf.in, pwscf.out - input/output files for pw.x | | | | |- job.sh - submission script | | | | | | | |- eq_pos_Ang_221.txt - txt file with the equilibrium geometrical and magnetic structure in the 2x2x1 supercell (needed by generate.sh) | | | |- displ_221.txt - txt file with the phonon displacements in the 2x2x1 supercell (needed by generate.sh) | | | |- generate.sh - bash script that 1) generates one folder for each amplitude of the displacement between -0.2 and 0.2, | | | | and inside it 2) generates the input files for the system in the distorted configurations due to | | | | the phonon displacement with that particular amplitude | | | | | |- collect_mag.sh - bash scipt that collects the final magnetic moments and check whether the initial spin configuration | | | was retained till the end of the electronic minimization or not | | | |** TEMPORAL_SERIES | | |** Conf* (*=1,...,11) (11 different spin configurations in the phonon-distorted 2x2x1 supercell needed for the calculation of the | | | | independent J parameters) | | | |** timepp_* (*=-0.0, ..., 10.0) (different time steps along the temporal series) | | | | |- pwscf.in, pwscf.out - input/output files for pw.x | | | | |- job.sh - submission script | | | | | | | |- eq_pos_Ang_221.txt - txt file with the equilibrium geometrical and magnetic structure in the 2x2x1 supercell (needed by generate.sh) | | | |- displ_***.txt - txt file with the 3 phonon displacementss in the 2x2x1 supercell that are combined along the | | | | temporal series (needed by generate.sh) | | | |- generate.sh - bash script that 1) generates one folder for each time step along the temporal series between 0.0 and 10 ps, | | | | and inside it 2) generates the input files for the system in the distorted configurations due to linear | | | | combination of the 3 involved phonon displacements | | | | | |- collect_mag.sh - bash scipt that collects the final magnetic moments and check whether the initial spin configuration | | | was retained till the end of the electronic minimization or not | pseudo (folder containing pseudopotentials. These are the pseudopotentials from the SSSP library https://www.materialscloud.org/discover/sssp/table/efficiency) |- Cu_pbe_v1.2.uspp.F.UPF |- O.pbe-n-kjpaw_psl.0.1.UPF |- Sr_pbe_v1.uspp.F.UPF |- b_pbe_v1.4.uspp.F.UPF