In this repository are attached the raw data related to the manuscript: Shape-controlled pathways in the hydrogen production from ethanol steam reforming over ceria nanoparticles ################################################################################################## The calculations were carried out using the slab−supercell approach, with the Vienna Ab-initio Simulation Program (VASP, http://www.vasp.at; version 5.4.4) All data is grouped into three .zip files: adsorbed_molecules.zip molecules_gas_phase.zip surfaces.zip Each directory found inside the zip files contains the following vasp inputs and outputs: INCAR.txt, CONTCAR.txt, OUTCAR.txt, KPOINTS.txt, POSCAR.txt, and OSZICAR.txt Description of the zip files - surfaces.zip: It contains the 5 ceria surface models as described in the manuscript. CeO2(111) --> CeO2(111) with 3x3 unit cell CeO2(100)-O --> CeO2(100) oxygen terminated with c(2x2) unit cell CeO2(100)-Mix --> CeO2(100) with a mixture of the O- and Ce- terminations (75% [(100)−O]-25% [(100)−Ce]) with c(2×2) unit cell Hydro-CeO2(100)-O --> Hydroxylated surface made of 3 dissociated water molecules on CeO2(100)-O Hydro-CeO2(100)-Mix --> Hydroxylated surface made of 3 dissociated water molecules on CeO2(100)-Mix - adsorbed_molecules.zip: It contains 13 folders with 10 kinds of ethoxy states, 2 ethylenedioxy and one ethylene on both surfaces of CeO2(111) and (100) and with different degree of hydroxylation. C2H5O-mI --> adsorbed monodentate standing up (SU) ethoxy on CeO2(111). C2H5O-mII --> adsorbed monodentate laying down (LD) ethoxy on CeO2(111). C2H5O-mIII --> adsorbed monodentate SU ethoxy on CeO2(100)-Mix. C2H5O-bd --> adsorbed bidentate ethoxy on CeO2(100)-O. C2H5O-mII-OHdiff --> same state as C2H5O-mII, but with an OH first-neighbour to the ethoxy. C2H5O-LD-CeO2(100) --> adsorbed monodentate LD ethoxy on the bare CeO2(100)-O. C2H5O-SU-CeO2(100) --> adsorbed monodentate SU ethoxy on the bare CeO2(100)-O. C2H5O-LD+H2O-CeO2(100) --> adsorbed monodentate LD ethoxy on the CeO2(100)-O with a dissociated water molecule. C2H5O-SU+H2O-CeO2(100) --> adsorbed monodentate SU ethoxy on the CeO2(100)-O with a dissociated water molecule. C2H5O-SU.1+3H2O-CeO2(100) --> adsorbed monodentate SU ethoxy on the CeO2(100)-O with 3 dissociated water molecules. This state es less stable than C2H5O-mIII. ethylene-CeO2(111) --> adsorbed ethylene on a rich hidroxylated environment on CeO2(111). ethylenedioxy-CeO2(111) --> adsorbed ethylenedioxy on a rich hidroxylated environment on CeO2(111). ethylenedioxy-CeO2(100) --> adsorbed ethylenedioxy on a rich hidroxylated environment on CeO2(100)-O. - molecules_gas_phase.zip: It contains the 2 folders with ethanol and water in the gas phase.