1. Fully optimized structures of graphene oxide (GO) nanosheets with different O/C ratios, obtained via the GFN2-xTB method in an implicit aqueous environment, for mean polarizability index (MPI) calculations. File format: xyz (1) O/C = 20%, GO20_optimized_coordinates.xyz (2) O/C = 30%, GO30_optimized_coordinates.xyz (3) O/C = 30%, GO30_optimized_coordinates.xyz 2. Optimized interaction structures of GO with different O/C ratios and solvent molecules (water, hexane, methanol), obtained via the GFN2-xTB method. File format: xyz (1). O/C = 20%, GO20-water.xyz (2). O/C = 20%, GO20-methanol.xyz (3). O/C = 20%, GO20-hexane.xyz (4). O/C = 30%, GO30-water.xyz (5). O/C = 30%, GO30-methanol.xyz (5). O/C = 30%, GO30-hexane.xyz (6). O/C = 40%, GO40-water.xyz (7). O/C = 40%, GO40-methanol.xyz (8). O/C = 40%, GO40-hexane.xyz 3. Initial and final snapshot configurations extracted from molecular dynamics (MD) simulation trajectories, showing the transport of single-component and mixed-component solvent molecules through GO interlayer nanochannels. Pure solvents: (1). Water (a). GO20-water_init_conf.gro (b). GO30-water_init_conf.gro (c). GO40-water_init_conf.gro (2). Methanol (a). GO20-methanol_init_conf.gro (b). GO30-methanol_init_conf.gro (c). GO40-methanol_init_conf.gro (3). Hexane (a). GO20-hexane_init_conf.gro (b). GO30-hexane_init_conf.gro (c). GO40-hexane_init_conf.gro Mixed solvents: (1). Water/methanol (95:5 mass ratio) (a). GO20_init_conf.gro (b). GO30_init_conf.gro (c). GO40_init_conf.gro (2). Methanol/hexane (95:5 mass ratio) (a). GO20_init_conf.gro (b). GO30_init_conf.gro (c). GO40_init_conf.gro