This database contains the results of: PBE cell optimization PBE HOMO and LUMO cubes PBE projected density of states files PBE triplet energy computation PBE triplet HOMO-alpha and LUMO-beta PBE electron injection (charge -1) doublet energy computation PBE electron injection (charge -1) HOMO-alpha PBE hole injection (charge +1) doublet energy computation PBE hole injection (charge +1) LUMO-beta PBE0 energy computation at PBE optimiwed geometry PBE0 excited states with tddft(tda) as implemented in CP2K (three lowest singlets) PBE0 HOMO and LUMO cubes PBE0 projected density of states files PBE0 triplet energy computation PBE0 triplet HOMO-alpha and LUMO-beta PBE0 electron injection (charge -1) doublet energy computation PBE0 electron injection (charge -1) HOMO-alpha PBE0 hole injection (charge +1) doublet energy computation PBE0 hole injection (charge +1) LUMO-beta BANDS structure computations at PBE level LAMBDA.xlsx file containing the computation of the charge separation values from the tddft(tda) coefficients and the spatial overlap. The 15-set of MOF studied are: AlPMOF MIL125 MIL125-NH2 MOF5 MOF5-NH2 MOF-74Zn MOFZn1 MUV11 NNU36 NTU-9 UiO66 UiO66-NH2 ZSTU-1 ZSTU-2 Zn2TTFB All computations have been done with CP2K version 6.1 See the "README" files inside each folder PBE, PBE0 and BANDS for more information about their contents.