In this repository are attached the raw data related to the manuscript: Dynamic Response of Oxygen Vacancies on the Deacon Reaction over Reduced Single Crystalline CeO2-x(111) Surfaces ################################################################################################## The calculations were carried out using the slab−supercell approach, with the Vienna Ab-initio Simulation Program (VASP, http://www.vasp.at; version 5.3.5 and 6.3.0) All data is grouped into three .zip files: Surfaces_Models.zip Chlorine_Adsorption.zip Hydrogen_Adsorption.zip Each directory found inside the zip files contains the following vasp inputs and outputs: INCAR.txt, CONTCAR.txt, OUTCAR.txt, KPOINTS.txt, POSCAR.txt, OSZICAR.txt and CONTCAR.jpg/png Description of the zip files - Surfaces_Models.zip: It contains the 5 ceria (111) surface models as described in the manuscript. CeO2.s3xs3 --> oxidized CeO2 with sqrt(3)xsqrt(3) unit cell CeO2-x.s3xs3 --> reduced CeO2, with 1 Oxygen vacancy, with sqrt(3)xsqrt(3) unit cell Ce7O12.s7xs7 --> reduced CeO2, with 1 Surface and 1 Subsurface Oxygen vacancies, with sqrt(7)xsqrt(7) unit cell Ce3O5.3x3 --> reduced CeO2, with 1 Surface and 2 Subsurface Oxygen vacancies, with 3x3 unit cell Ce2O3-CeO2.4x4 --> reduced CeO2 with a quintuple layer of Ce2O3 and a 4x4 unit cell - Chlorine_Adsorption.zip: It contains the 5 folders with Cl atoms adsorbed in the different models. 1Cl.CeO2.s3xs3 --> 1Cl atom adsorbed on CeO2.s3xs3 1Cl.CeO2-x.s3xs3 --> 1Cl atom adsorbed on CeO2-x.s3xs3 2Cl.Ce7O12.s7xs7 --> 2Cl atoms adsorbed on Ce7O12.s7xs7 3Cl.Ce3O5.3x3 --> 3Cl atoms adsorbed on Ce3O5.3x3 5Cl.Ce2O3-CeO2.4x4 --> 5Cl atoms adsorbed on Ce2O3-CeO2.4x4 - Hydrogen_Adsorption.zip: It contains the 3 folders with H atoms adsorbed in the different models. 2H.Ce7O12.s7xs7 --> 2H atoms adsorbed on Ce7O12.s7xs7 3H.Ce3O5.3x3 --> 3H atoms adsorbed on Ce3O5.3x3 5H.Ce2O3-CeO2.4x4 --> 5H atoms adsorbed on Ce2O3-CeO2.4x4