All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle


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{
  "created": "2023-06-05T09:18:16.193129+00:00", 
  "metadata": {
    "references": [
      {
        "citation": "R. Zeng, L. Zhu, M. Zhang, W. Zhong, G. Zhou, J. Zhuang, T. Hao, Z. Zhou, L. Zhou, N. Hartmann, X. Xue, H. Jing, F. Han, Y. Bai, H. Wu, Z. Tang, Y. Zou, H. Zhu, C. Chen, Y. Zhang, F. Liu, nat. commun. 14, 4148 (2023)", 
        "comment": "Paper in which the method is described", 
        "doi": "https://doi.org/10.1038/s41467-023-39832-4", 
        "type": "Journal reference"
      }
    ], 
    "mcid": "2023.89", 
    "id": "1787", 
    "is_last": true, 
    "title": "All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle", 
    "publication_date": "Jun 07, 2023, 10:57:52", 
    "edited_by": 1048, 
    "_oai": {
      "id": "oai:materialscloud.org:1787"
    }, 
    "version": 1, 
    "description": "Distributed photovoltaics in living environment harvest the sunlight in different incident angles throughout the day. The development of planer solar cells with large light-receiving angle can reduce the requirements in installation form factor and is therefore urgently required. Here, thin film organic photovoltaics with nano-sized phase separation integrated in micro-sized surface topology is demonstrated as an ideal solution to proposed applications. All-polymer solar cells, by means of a newly developed sequential processing, show large magnitude hierarchical morphology with facilitated exciton-to-carrier conversion. The nano fibrilar donor-acceptor network and micron-scale optical field trapping structure in combination contributes to an efficiency of 19.06% (certified 18.59%), which is the highest value to date for all-polymer solar cells. Furthermore, the micron-sized surface topology also contributes to a large light-receiving angle. A 30% improvement of power gain is achieved for the hierarchical morphology comparing to the flat-morphology devices. These inspiring results show that all-polymer solar cell with hierarchical features are particularly suitable for the commercial applications of distributed photovoltaics due to its low installation requirement.", 
    "status": "published", 
    "license_addendum": null, 
    "keywords": [
      "organic solar cells", 
      "all-polymer solar cell", 
      "surface topology"
    ], 
    "license": "Creative Commons Attribution 4.0 International", 
    "owner": 1048, 
    "contributors": [
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zeng", 
        "givennames": "Rui"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhu", 
        "givennames": "Lei"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhang", 
        "givennames": "Ming"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhong", 
        "givennames": "Wenkai"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhou", 
        "givennames": "Guanqing"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhuang", 
        "givennames": "Jiaxing"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Hao", 
        "givennames": "Tianyu"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhou", 
        "givennames": "Zichun"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhou", 
        "givennames": "Libo"
      }, 
      {
        "affiliations": [
          "Attocube systems AG, Eglfinger Weg 2, Haar 85540, Germany."
        ], 
        "familyname": "Hartmann", 
        "givennames": "Nicolai"
      }, 
      {
        "affiliations": [
          "Shanghai OPV Solar New Energy Technology Co., Ltd., Shanghai 201210, China."
        ], 
        "familyname": "Xue", 
        "givennames": "Xiaonan"
      }, 
      {
        "affiliations": [
          "Shanghai OPV Solar New Energy Technology Co., Ltd., Shanghai 201210, China."
        ], 
        "familyname": "Jing", 
        "givennames": "Hao"
      }, 
      {
        "affiliations": [
          "State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources, North China Electric Power University, Beijing 102206, China."
        ], 
        "familyname": "Han", 
        "givennames": "Fei"
      }, 
      {
        "affiliations": [
          "State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources, North China Electric Power University, Beijing 102206, China."
        ], 
        "familyname": "Bai", 
        "givennames": "Yiming"
      }, 
      {
        "affiliations": [
          "Center for Advanced Low-dimension Materials, State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering Donghua University, Shanghai 201620, China"
        ], 
        "familyname": "Wu", 
        "givennames": "Hongbo"
      }, 
      {
        "affiliations": [
          "Center for Advanced Low-dimension Materials, State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering Donghua University, Shanghai 201620, China"
        ], 
        "familyname": "Tang", 
        "givennames": "Zheng"
      }, 
      {
        "affiliations": [
          "State Key Laboratory of Fluorinated Functional Membrane Materials and Dongyue Future Hydrogen Energy Materials Company, Zibo City, Shandong 256401, China."
        ], 
        "familyname": "Zou", 
        "givennames": "Yecheng"
      }, 
      {
        "affiliations": [
          "Department of Chemistry, Zhejiang University, Hangzhou, Zhejiang 310027, China."
        ], 
        "familyname": "Zhu", 
        "givennames": "Haiming"
      }, 
      {
        "affiliations": [
          "School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Chen", 
        "givennames": "Chun-chao"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Zhang", 
        "givennames": "Yongming"
      }, 
      {
        "affiliations": [
          "School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
        ], 
        "familyname": "Liu", 
        "email": "fengliu82@sjtu.edu.cn", 
        "givennames": "Feng"
      }
    ], 
    "conceptrecid": "1786", 
    "doi": "10.24435/materialscloud:g4-jw", 
    "_files": [
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        "size": 37660, 
        "key": "Figure2.xlsx", 
        "description": "Photo-electric performance and statistics of all polymer solar cells.", 
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        "key": "Figure3.xlsx", 
        "description": "The data of nanoscale fibril crystallization morphology characteristics for all polymer solar cells.", 
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        "key": "Figure4.xlsx", 
        "description": "The performance comparison for all polymer solar cells at different light receiving angle based on microscale surface optical morphology.", 
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        "description": "Dissociation and recombination dynamics results based on ultrafast process and devices physical characteristics.", 
        "checksum": "md5:d546e32136be8079502884c15943f1f1"
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        "size": 14686, 
        "key": "Table 1.xlsx", 
        "description": "Specific performance parameters in different preparation conditions based on all polymer solar cells.", 
        "checksum": "md5:2c26dd4f98b3ddc0c5bc4ccf7b73387d"
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        "key": "Supplementary Table.xlsx", 
        "description": "Specific parameters for morphology characterization and device characterization in Supplementary Tables.", 
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        "key": "Supplementary Figure.xlsx", 
        "description": "Other relevant data in Supplementary Figures.", 
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    ]
  }, 
  "id": "1787", 
  "updated": "2023-07-13T07:46:12.140992+00:00", 
  "revision": 6
}