All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle
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{
"id": "1787",
"updated": "2023-07-13T07:46:12.140992+00:00",
"metadata": {
"version": 1,
"contributors": [
{
"givennames": "Rui",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zeng"
},
{
"givennames": "Lei",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhu"
},
{
"givennames": "Ming",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhang"
},
{
"givennames": "Wenkai",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhong"
},
{
"givennames": "Guanqing",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhou"
},
{
"givennames": "Jiaxing",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhuang"
},
{
"givennames": "Tianyu",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Hao"
},
{
"givennames": "Zichun",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhou"
},
{
"givennames": "Libo",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhou"
},
{
"givennames": "Nicolai",
"affiliations": [
"Attocube systems AG, Eglfinger Weg 2, Haar 85540, Germany."
],
"familyname": "Hartmann"
},
{
"givennames": "Xiaonan",
"affiliations": [
"Shanghai OPV Solar New Energy Technology Co., Ltd., Shanghai 201210, China."
],
"familyname": "Xue"
},
{
"givennames": "Hao",
"affiliations": [
"Shanghai OPV Solar New Energy Technology Co., Ltd., Shanghai 201210, China."
],
"familyname": "Jing"
},
{
"givennames": "Fei",
"affiliations": [
"State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources, North China Electric Power University, Beijing 102206, China."
],
"familyname": "Han"
},
{
"givennames": "Yiming",
"affiliations": [
"State Key Laboratory of Alternate Electrical Power System with Renewable Energy Sources, North China Electric Power University, Beijing 102206, China."
],
"familyname": "Bai"
},
{
"givennames": "Hongbo",
"affiliations": [
"Center for Advanced Low-dimension Materials, State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering Donghua University, Shanghai 201620, China"
],
"familyname": "Wu"
},
{
"givennames": "Zheng",
"affiliations": [
"Center for Advanced Low-dimension Materials, State Key Laboratory for Modification of Chemical Fibers and Polymer Materials, College of Materials Science and Engineering Donghua University, Shanghai 201620, China"
],
"familyname": "Tang"
},
{
"givennames": "Yecheng",
"affiliations": [
"State Key Laboratory of Fluorinated Functional Membrane Materials and Dongyue Future Hydrogen Energy Materials Company, Zibo City, Shandong 256401, China."
],
"familyname": "Zou"
},
{
"givennames": "Haiming",
"affiliations": [
"Department of Chemistry, Zhejiang University, Hangzhou, Zhejiang 310027, China."
],
"familyname": "Zhu"
},
{
"givennames": "Chun-chao",
"affiliations": [
"School of Materials Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Chen"
},
{
"givennames": "Yongming",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"familyname": "Zhang"
},
{
"givennames": "Feng",
"affiliations": [
"School of Chemistry and Chemical Engineering, Frontiers Science Center for Transformative Molecules, In-situ Center for Physical Science, and Center of Hydrogen Science Shanghai Jiao Tong University, Shanghai 200240, China."
],
"email": "fengliu82@sjtu.edu.cn",
"familyname": "Liu"
}
],
"title": "All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle",
"_oai": {
"id": "oai:materialscloud.org:1787"
},
"keywords": [
"organic solar cells",
"all-polymer solar cell",
"surface topology"
],
"publication_date": "Jun 07, 2023, 10:57:52",
"_files": [
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"key": "Figure2.xlsx",
"description": "Photo-electric performance and statistics of all polymer solar cells.",
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"key": "Figure3.xlsx",
"description": "The data of nanoscale fibril crystallization morphology characteristics for all polymer solar cells.",
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{
"key": "Figure4.xlsx",
"description": "The performance comparison for all polymer solar cells at different light receiving angle based on microscale surface optical morphology.",
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"key": "Figure5.xlsx",
"description": "Dissociation and recombination dynamics results based on ultrafast process and devices physical characteristics.",
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{
"key": "Table 1.xlsx",
"description": "Specific performance parameters in different preparation conditions based on all polymer solar cells.",
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{
"key": "Supplementary Table.xlsx",
"description": "Specific parameters for morphology characterization and device characterization in Supplementary Tables.",
"checksum": "md5:cda177f998f4a98285a049c3344ff817",
"size": 67310
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{
"key": "Supplementary Figure.xlsx",
"description": "Other relevant data in Supplementary Figures.",
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"references": [
{
"comment": "Paper in which the method is described",
"doi": "https://doi.org/10.1038/s41467-023-39832-4",
"citation": "R. Zeng, L. Zhu, M. Zhang, W. Zhong, G. Zhou, J. Zhuang, T. Hao, Z. Zhou, L. Zhou, N. Hartmann, X. Xue, H. Jing, F. Han, Y. Bai, H. Wu, Z. Tang, Y. Zou, H. Zhu, C. Chen, Y. Zhang, F. Liu, nat. commun. 14, 4148 (2023)",
"type": "Journal reference"
}
],
"description": "Distributed photovoltaics in living environment harvest the sunlight in different incident angles throughout the day. The development of planer solar cells with large light-receiving angle can reduce the requirements in installation form factor and is therefore urgently required. Here, thin film organic photovoltaics with nano-sized phase separation integrated in micro-sized surface topology is demonstrated as an ideal solution to proposed applications. All-polymer solar cells, by means of a newly developed sequential processing, show large magnitude hierarchical morphology with facilitated exciton-to-carrier conversion. The nano fibrilar donor-acceptor network and micron-scale optical field trapping structure in combination contributes to an efficiency of 19.06% (certified 18.59%), which is the highest value to date for all-polymer solar cells. Furthermore, the micron-sized surface topology also contributes to a large light-receiving angle. A 30% improvement of power gain is achieved for the hierarchical morphology comparing to the flat-morphology devices. These inspiring results show that all-polymer solar cell with hierarchical features are particularly suitable for the commercial applications of distributed photovoltaics due to its low installation requirement.",
"status": "published",
"license": "Creative Commons Attribution 4.0 International",
"conceptrecid": "1786",
"is_last": true,
"mcid": "2023.89",
"edited_by": 1048,
"id": "1787",
"owner": 1048,
"license_addendum": null,
"doi": "10.24435/materialscloud:g4-jw"
},
"revision": 6,
"created": "2023-06-05T09:18:16.193129+00:00"
}