All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle


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<oai_dc:dc xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:oai_dc="http://www.openarchives.org/OAI/2.0/oai_dc/" xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xsi:schemaLocation="http://www.openarchives.org/OAI/2.0/oai_dc/ http://www.openarchives.org/OAI/2.0/oai_dc.xsd">
  <dc:creator>Zeng, Rui</dc:creator>
  <dc:creator>Zhu, Lei</dc:creator>
  <dc:creator>Zhang, Ming</dc:creator>
  <dc:creator>Zhong, Wenkai</dc:creator>
  <dc:creator>Zhou, Guanqing</dc:creator>
  <dc:creator>Zhuang, Jiaxing</dc:creator>
  <dc:creator>Hao, Tianyu</dc:creator>
  <dc:creator>Zhou, Zichun</dc:creator>
  <dc:creator>Zhou, Libo</dc:creator>
  <dc:creator>Hartmann, Nicolai</dc:creator>
  <dc:creator>Xue, Xiaonan</dc:creator>
  <dc:creator>Jing, Hao</dc:creator>
  <dc:creator>Han, Fei</dc:creator>
  <dc:creator>Bai, Yiming</dc:creator>
  <dc:creator>Wu, Hongbo</dc:creator>
  <dc:creator>Tang, Zheng</dc:creator>
  <dc:creator>Zou, Yecheng</dc:creator>
  <dc:creator>Zhu, Haiming</dc:creator>
  <dc:creator>Chen, Chun-chao</dc:creator>
  <dc:creator>Zhang, Yongming</dc:creator>
  <dc:creator>Liu, Feng</dc:creator>
  <dc:date>2023-06-07</dc:date>
  <dc:description>Distributed photovoltaics in living environment harvest the sunlight in different incident angles throughout the day. The development of planer solar cells with large light-receiving angle can reduce the requirements in installation form factor and is therefore urgently required. Here, thin film organic photovoltaics with nano-sized phase separation integrated in micro-sized surface topology is demonstrated as an ideal solution to proposed applications. All-polymer solar cells, by means of a newly developed sequential processing, show large magnitude hierarchical morphology with facilitated exciton-to-carrier conversion. The nano fibrilar donor-acceptor network and micron-scale optical field trapping structure in combination contributes to an efficiency of 19.06% (certified 18.59%), which is the highest value to date for all-polymer solar cells. Furthermore, the micron-sized surface topology also contributes to a large light-receiving angle. A 30% improvement of power gain is achieved for the hierarchical morphology comparing to the flat-morphology devices. These inspiring results show that all-polymer solar cell with hierarchical features are particularly suitable for the commercial applications of distributed photovoltaics due to its low installation requirement.</dc:description>
  <dc:identifier>https://archive.materialscloud.org/record/2023.89</dc:identifier>
  <dc:identifier>doi:10.24435/materialscloud:g4-jw</dc:identifier>
  <dc:identifier>mcid:2023.89</dc:identifier>
  <dc:identifier>oai:materialscloud.org:1787</dc:identifier>
  <dc:language>en</dc:language>
  <dc:publisher>Materials Cloud</dc:publisher>
  <dc:rights>info:eu-repo/semantics/openAccess</dc:rights>
  <dc:rights>Creative Commons Attribution 4.0 International https://creativecommons.org/licenses/by/4.0/legalcode</dc:rights>
  <dc:subject>organic solar cells</dc:subject>
  <dc:subject>all-polymer solar cell</dc:subject>
  <dc:subject>surface topology</dc:subject>
  <dc:title>All-polymer organic solar cells with nano-to-micron hierarchical morphology and large light receiving angle</dc:title>
  <dc:type>Dataset</dc:type>
</oai_dc:dc>