Disorder-resilient transition of Helical to Conical ground states in M<sub>1/3</sub>NbS<sub>2</sub>, M=Cr,Mn
JSON Export
{
"revision": 2,
"id": "2547",
"created": "2025-01-28T08:59:08.906971+00:00",
"metadata": {
"doi": "10.24435/materialscloud:qa-5v",
"status": "published",
"title": "Disorder-resilient transition of Helical to Conical ground states in M<sub>1/3</sub>NbS<sub>2</sub>, M=Cr,Mn",
"mcid": "2025.20",
"license_addendum": null,
"_files": [
{
"description": "Experimental data and input/output files for the simulations appearing in the manuscript.",
"key": "MNb3S6_data_v2.tgz",
"size": 35856259,
"checksum": "md5:5cfe9845a33ec9aaf5c4cd6461d04baa"
}
],
"owner": 80,
"_oai": {
"id": "oai:materialscloud.org:2547"
},
"keywords": [
"Chiral Helical Magnetism",
"Nuclear Magnetic Resonance",
"DFT",
"Chiral Soliton Lattice"
],
"conceptrecid": "2289",
"is_last": true,
"references": [
{
"type": "Preprint",
"doi": "10.48550/arXiv.2410.01631",
"url": "http://arxiv.org/abs/2410.01631",
"citation": "M. Sahoo, P. Bonf\u00e0, A. E. Hall, D. A. Mayoh, L. T. Corredor, A. U. B Wolter, B. B\u00fcchner, G. Balakrishnan, R. De Renzi, G. Allodi, arXiv:2410.01631"
}
],
"publication_date": "Jan 28, 2025, 12:08:17",
"license": "Creative Commons Attribution 4.0 International",
"id": "2547",
"description": "The discovery of chiral helical magnetism (CHM) in Cr<sub>1/3</sub>NbS<sub>2</sub> and the stabilization of a chiral soliton lattice (CSL) has attracted considerable interest in view of their potential technological applications. However, there is an ongoing debate regarding whether the sister compound, Mn<sub>1/3</sub>NbS<sub>2</sub>, which shares the same crystal structure, exhibits similar nontrivial properties, which rely on the stabilization of the lack of inversion symmetry at the magnetic ion. In this study, we conduct a comprehensive investigation of the magnetically ordered states of both compounds, using <sup>53</sup>Cr, <sup>55</sup>Mn and <sup>93</sup>Nb nuclear magnetic resonance. Our results, supported by density functional calculations, detect in a high quality single crystal of Cr<sub>1/3</sub>NbS<sub>2</sub> all the signatures of the monoaxial CHM in a magnetic field, identifying it as a textbook NMR case. The detailed understanding of this prototypic behavior provides a reference for Mn<sub>1/3</sub>NbS<sub>2</sub>.\nDespite the much larger density of specific defects in this second single crystal, we confirm the presence of a CHM phase in the Mn compound, characterized by a very large critical field for the forced ferromagnetic phase (~ 10 T for H || c).",
"version": 2,
"contributors": [
{
"email": "manaswinisahoo333@gmail.com",
"affiliations": [
"Dipartimento di Scienze Matematiche, Fisiche e Informatiche, Universit\u00e0 di Parma, Parco Area delle Scienze 7/A, I-43124 Parma, Italy",
"Leibniz IFW Dresden, Helmholtzstrasse 20, D-01069 Dresden, Germany",
"Institut f\u00fcr Festk\u00f6rper- und Materialphysik, Technische Universit\u00e4t Dresden, 01062 Dresden, Germany"
],
"familyname": "Sahoo",
"givennames": "Manaswini"
},
{
"email": "pietro.bonfa@unipr.it",
"affiliations": [
"Dipartimento di Scienze Matematiche, Fisiche e Informatiche, Universit\u00e0 di Parma, Parco Area delle Scienze 7/A, I-43124 Parma, Italy"
],
"familyname": "Bonf\u00e0",
"givennames": "Pietro"
},
{
"affiliations": [
"Department of Physics, University of Warwick, Coventry, CV4 7AL, United Kingdom"
],
"familyname": "Hall",
"givennames": "Amelia Elisabeth"
},
{
"affiliations": [
"Department of Physics, University of Warwick, Coventry, CV4 7AL, United Kingdom"
],
"familyname": "Mayoh",
"givennames": "Daniel A."
},
{
"affiliations": [
"Leibniz IFW Dresden, Helmholtzstrasse 20, D-01069 Dresden, Germany"
],
"familyname": "Corredor",
"givennames": "Laura Teresa"
},
{
"affiliations": [
"Leibniz IFW Dresden, Helmholtzstrasse 20, D-01069 Dresden, Germany"
],
"familyname": "Wolter",
"givennames": "Anja U. B."
},
{
"affiliations": [
"Leibniz IFW Dresden, Helmholtzstrasse 20, D-01069 Dresden, Germany"
],
"familyname": "B\u00fcchner",
"givennames": "Bernd"
},
{
"affiliations": [
"Department of Physics, University of Warwick, Coventry, CV4 7AL, United Kingdom"
],
"familyname": "Balakrishnan",
"givennames": "Geetha"
},
{
"affiliations": [
"Dipartimento di Scienze Matematiche, Fisiche e Informatiche, Universit\u00e0 di Parma, Parco Area delle Scienze 7/A, I-43124 Parma, Italy"
],
"familyname": "De Renzi",
"givennames": "Roberto"
},
{
"affiliations": [
"Dipartimento di Scienze Matematiche, Fisiche e Informatiche, Universit\u00e0 di Parma, Parco Area delle Scienze 7/A, I-43124 Parma, Italy"
],
"familyname": "Allodi",
"givennames": "Giuseppe"
}
],
"edited_by": 576
},
"updated": "2025-01-28T11:08:17.805088+00:00"
}