Published May 5, 2026 | Version v1
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Characteristic data of activation of crystalline and amorphous OER catalysts with bulk and surface Fe incorporation.

  • 1. PSI Center for Energy and Environmental Science, 5232 Villigen PSI, Switzerland
  • 2. ROR icon ETH Zurich

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Description

This electrochemical, X-ray diffraction, and operando X-ray abosorption spectroscopy data characterize and decouple the effects of bulk vs. electrolyte Fe incorporation in crystalline, defective crystalline, and amorphous catalysts derived from the same CoSn(OH)₆ precursor. Electrolyte Fe incorporation equalizes the OER activity across all three structural variants, demonstrating that surface Fe chemistry can dominate initial structural effects on the reconstructed catalyst interface.

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Funding

Swiss National Science Foundation
PRIMA PR00P2_193111

References

Journal reference (UNDER REVIEW; Paper in which the electrochemical activation, characterization methods, and structure-activity trends are described in detail.)
K. Crossley, J. Grotheer, J. Huang, T.J. Schmidt, E. Fabbri. Advanced Energy and Sustainability Research, (UNDER REVIEW, 2026)